B16-Test Beamline
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M.
Borri
,
C.
Cohen
,
O.
Fox
,
J.
Groves
,
W.
Helsby
,
O.
Mathon
,
L.
Mcnicholl
,
S.
Pascarelli
,
K.
Sawhney
,
R.
Torchio
,
M.
Zuvic
Diamond Proposal Number(s):
[24637]
Open Access
Abstract: Germanium micro-strip sensors were selected as the sensor technology to take data in energy dispersive X-ray spectroscopy experiments at the Extremely Brilliant Source (EBS) in Grenoble (FR). It is important for this experimental technique to use sensors with a large uniform area and a fine pitch. The former determines the range of energy detectable with a single sensor. The latter improves spectral resolution. A high stopping power is also important to perform studies with hard X-rays.
The device under test in this measurement was a germanium micro-strip sensor made of 1024 strips with
pitch. The bulk was 1.5 mm thick. The sensor was assembled into a prototype cryostat part of the XH detector system. The device was tested at the B16 beamline at the Diamond Light Source (DLS) in Didcot (UK). The objective of the test-beam was to characterise charge-sharing between strips. In fact, this effect limits the spectral resolution of the device.
To carry out this test, the sensor was scanned over a subset of strips with micro-focused X-rays under different settings. These were beam energy and intensity, sensor temperature and bias voltage. Results are presented in this paper. It was measured that the full width half maximum of the charge-sharing profile across different strips was
for settings which were indicative of the experimental conditions at the EBS. This was a signal current per unit area on the sensor of
10−8 A/
, a bias voltage of -180 V and a temperature of -159
C.
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Dec 2020
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B16-Test Beamline
B18-Core EXAFS
I08-Scanning X-ray Microscopy beamline (SXM)
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Debi
Garai
,
Vladyslav
Solokha
,
Axel
Wilson
,
Ilaria
Carlomagno
,
Ajay
Gupta
,
Mukul
Gupta
,
V. R.
Reddy
,
Carlo
Meneghini
,
Francesco
Carla
,
Christian
Morawe
,
Jorg
Zegenhagen
Diamond Proposal Number(s):
[17145]
Open Access
Abstract: This work reports about a novel approach for investigating surface processes during the early stages of galvanic corrosion of stainless steel in situ by employing ultra-thin films and synchrotron X-radiation. Characterized by X-ray techniques and voltammetry, such films, sputter deposited from austenitic steel, were found representing useful replicas of the target material. Typical for stainless steel, the surface consists of a passivation layer of Fe- and Cr-oxides, a couple of nm thick, that is depleted of Ni. Films of ≈ 4 nm thickness were studied in situ in an electrochemical cell under potential control (-0.6 to +0.8 V vs Ag/AgCl) during exposure to 0.1 M KCl. Material transport was recorded with better than 1/10 monolayer sensitivity by X-ray spectroscopy. Leaching of Fe was observed in the cathodic range and the therefor necessary reduction of Fe-oxide appears to be accelerated by atomic hydrogen. Except for minor leaching, reduction of Ni, while expected from Pourbaix diagram, was not observed until at ≈ +0.8 V Cr-oxide was removed from the film. After couple of minutes exposure at +0.8 V, the current in the electrochemical cell revealed a rapid pitting event that was simultaneously monitored by X-ray spectroscopy. Continuous loss of Cr and Ni was observed during the induction time leading to the pitting, suggesting a causal connection with the event. Finally, a spectroscopic image of a pit was recorded ex situ with 50 nm lateral and 1 nm depth resolution by soft X-ray scanning absorption microscopy at the Fe L2,3-edges by using a 80 nm film on a SiN membrane, which is further demonstrating the usefulness of thin films for corrosion studies.
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Dec 2020
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B16-Test Beamline
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Abstract: The research topic of this thesis is related to cancer, which is a major health problem of the population and thus one of the leading causes of mortality worldwide, especially in highly urbanized and industrialized environments. Starting from disease-related statistics, through cancer treatment strategies including platinum-based anticancer drugs, we reach metal-based chemotherapy, highlighting the iron (Fe), copper (Cu) and zinc (Zn) based chelators and complexes, as well as their anticancer activity. In addition, the related drug delivery systems, especially the relevant literature on copper containing liposomes, is briefly summarized.
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Dec 2020
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B16-Test Beamline
Optics
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Open Access
Abstract: Ptychography is a scanning coherent diffraction imaging technique which provides high resolution imaging and complete spatial information of the complex electric field probe and sample transmission function. Its ability to accurately determine the illumination probe has led to its use at modern synchrotrons and free-electron lasers as a wavefront-sensing technique for optics alignment, monitoring and correction. Recent developments in the ptychography reconstruction process now incorporate a modal decomposition of the illuminating probe and relax the restriction of using sources with high spatial coherence. In this article a practical implementation of hard X-ray ptychography from a partially coherent X-ray source with a large number of modes is demonstrated experimentally. A strongly diffracting Siemens star test sample is imaged using the focused beam produced by either a Fresnel zone plate or beryllium compound refractive lens. The recovered probe from each optic is back propagated in order to plot the beam caustic and determine the precise focal size and position. The power distribution of the reconstructed probe modes also allows the quantification of the beams coherence and is compared with the values predicted by a Gaussian–Schell model and the optics exit intensity.
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Nov 2020
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B16-Test Beamline
Optics
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Open Access
Abstract: A refractive phase corrector optics is proposed for the compensation of fabrication error of X-ray optical elements. Here, at-wavelength wavefront measurements of the focused X-ray beam by knife-edge imaging technique, the design of a three-dimensional corrector plate, its fabrication by 3D printing, and use of a corrector to compensate for X-ray lens figure errors are presented. A rotationally invariant corrector was manufactured in the polymer IP-STM using additive manufacturing based on the two-photon polymerization technique. The fabricated corrector was characterized at the B16 Test beamline, Diamond Light Source, UK, showing a reduction in r.m.s. wavefront error of a Be compound refractive Lens (CRL) by a factor of six. The r.m.s. wavefront error is a figure of merit for the wavefront quality but, for X-ray lenses, with significant X-ray absorption, a form of the r.m.s. error with weighting proportional to the transmitted X-ray intensity has been proposed. The knife-edge imaging wavefront-sensing technique was adapted to measure rotationally variant wavefront errors from two different sets of Be CRL consisting of 98 and 24 lenses. The optical aberrations were then quantified using a Zernike polynomial expansion of the 2D wavefront error. The compensation by a rotationally invariant corrector plate was partial as the Be CRL wavefront error distribution was found to vary with polar angle indicating the presence of non-spherical aberration terms. A wavefront correction plate with rotationally anisotropic thickness is proposed to compensate for anisotropy in order to achieve good focusing by CRLs at beamlines operating at diffraction-limited storage rings.
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Nov 2020
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B16-Test Beamline
I15-Extreme Conditions
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Diamond Proposal Number(s):
[17704, 17707]
Open Access
Abstract: Purpose: Photon-counting silicon strip detectors are attracting interest for use in next-generation CT scanners. For CT detectors in a clinical environment, it is desirable to have a low power consumption. However, decreasing the power consumption leads to higher noise. This is particularly detrimental for silicon detectors, which require a low noise floor to obtain a good dose efficiency. The increase in noise can be mitigated using a longer shaping time in the readout electronics. This also results in longer pulses, which requires an increased deadtime, thereby degrading the count-rate performance. However, as the photon flux varies greatly during a typical CT scan, not all projection lines require a high count-rate capability. We propose adjusting the shaping time to counteract the increased noise that results from decreasing the power consumption.
Approach: To show the potential of increasing the shaping time to decrease the noise level, synchrotron measurements were performed using a detector prototype with two shaping time settings. From the measurements, a simulation model was developed and used to predict the performance of a future channel design.
Results: Based on the synchrotron measurements, we show that increasing the shaping time from 28.1 to 39.4 ns decreases the noise and increases the signal-to-noise ratio with 6.5% at low count rates. With the developed simulation model, we predict that a 50% decrease in power can be attained in a proposed future detector design by increasing the shaping time with a factor of 1.875.
Conclusion: Our results show that the shaping time can be an important tool to adapt the pulse length and noise level to the photon flux and thereby optimize the dose efficiency of photon-counting silicon detectors.
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Oct 2020
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B16-Test Beamline
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Antonino
Buttacavoli
,
Fabio
Principato
,
Gaetano
Gerardi
,
Manuele
Bettelli
,
Nicola
Sarzi Amade
,
Andrea
Zappettini
,
Paul
Seller
,
Matthew C.
Veale
,
Oliver
Fox
,
Kawal
Sawhney
,
Leonardo
Abbene
Diamond Proposal Number(s):
[20545]
Abstract: Cadmium–zinc–telluride (CZT) pixel detectors represent a consolidated choice for the development of room-temperature spectroscopic X-ray imagers, finding important applications in medical imaging, often as detection modules of a variety of new SPECT and CT systems. Detectors with 3–5 mm thicknesses are able to efficiently detect X-rays up to 140 keV giving reasonable room-temperature energy resolution. In this work, the room-temperature performance of 3 mm-thick CZT pixel detectors, recently developed at IMEM/CNR of Parma (Italy), is presented. Sub-millimetre detector arrays with pixel pitch less than 500 µm were fabricated. The detectors are characterized by good room-temperature performance even at high bias voltage operation (6000 V cm−1), with energy resolutions (FWHM) of 3% (1.8 keV) and 1.6% (2 keV) at 59.5 keV and 122.1 keV, respectively. Charge-sharing investigations were performed with both uncollimated and collimated synchrotron X-ray beams with particular attention to recovering the charge losses at the inter-pixel gap region. High rate measurements demonstrated the absence of high-flux radiation-induced polarization phenomena up to 25 × 106 photons mm−2 s−1.
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Sep 2020
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B16-Test Beamline
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S.
Santpur
,
A. J.
Blue
,
C.
Buttar
,
V.
Fadeyev
,
B.
Gallop
,
C.
Helling
,
C.
Labitan
,
P. W.
Phillips
,
L.
Poley
,
C.
Sawyer
,
M.
Ullán
,
Y.
Unno
Diamond Proposal Number(s):
[18807, 22002]
Abstract: Silicon strip sensors for the ATLAS Inner Tracker (ITk) have been designed to provide reliable particle detection in the high-radiation environment of the High-Luminosity Large Hadron Collider. One important design criterion for their development is the minimization of inactive sensor areas, which affect the hermiticity of particle detection inside the detector. In previous measurements of ATLAS silicon strip sensors, the charge-collecting area of individual strip implants has been mapped and found to agree with the sensor strip pitch and strip length. For strip implants next to the sensor bias ring, the extent of their charge-collecting area towards the inactive sensor area was previously unknown, which limited the accuracy of both overall detector hermiticity estimates and the position resolution for particle detection at the sensor edge. Therefore, measurements were conducted to map the area of charge collection for sensor strips at the edge of the active sensor area using a micro-focused X-ray beam. This publication presents measurements showing the extent of charge collection in the edge strips of silicon strip sensors for two generations of ATLAS ITk strip sensor modules. The measurements confirmed that charge deposited in a strip implant that is neither connected nor grounded leads to capacitive coupling to the adjacent strip, where it is indistinguishable from a hit in that strip.
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Sep 2020
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B16-Test Beamline
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Diamond Proposal Number(s):
[23604]
Open Access
Abstract: We demonstrate experimentally the ability to use a single-pixel detector for two-dimensional high-resolution x-ray imaging of fast dynamics. We image the rotation of a spinning chopper at 100 kHz and at spatial resolution of about 40 microns by using the computational ghost imaging approach. The technique we develop can be used for the imaging of fast dynamics of periodic and periodically stimulated effects with a large field of view and at low dose.
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Aug 2020
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B16-Test Beamline
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Diamond Proposal Number(s):
[21419]
Open Access
Abstract: Bone is a natural hierarchical composite tissue incorporating hard mineral nano-crystals of hydroxyapatite (HAp) and organic binding material containing elastic collagen fibers. In the study, we investigated the structure and deformation of ovine bone by the combination of high-energy synchrotron X-ray tomographic imaging and scattering. X-ray experiments were performed prior to and under three-point bending loading by using a specially developed in situ load cell constructed from aluminium alloy frame, fast-drying epoxy resin for sample fixation, and a titanium bolt for contact loading. Firstly, multiple radiographic projection images were acquired and tomographic reconstruction was performed using SAVU software, following segmentation using Avizo. Secondly, Wide Angle X-ray Scattering (WAXS) and Small Angle X-ray Scattering (SAXS) 2D scattering patterns were collected from HAp and collagen. Both sample shape and deformation affect the observed scattering. Novel combined tomographic and diffraction analysis presented below paves the way for advanced characterization of complex shape samples using the Dual Imaging and Diffraction (DIAD) paradigm.
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Aug 2020
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