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E01-JEM ARM 200CF	Evaluation and realization of safer Mg-S battery: the decisive role of the electrolyte Lin Sheng , Zhangxiang Hao , Junrun Feng , Wenjia Du , Manxi Gong , Liqun Kang , Paul R. Shearing , Dan J. I. Brett , Yunhui Huang , Feng Ryan Wang Nano Energy 334 DOI: 10.1016/j.nanoen.2021.105832 Diamond Proposal Number(s): [20643] Show Abstract ▼ Abstract: The magnesium–sulfur (Mg-S) battery may be a safer alternative for the lithium-sulfur battery because Mg plating usually proceeds without dendrite formation. Here, we correlate the thermal runaway of Mg-S battery with the associated change of electrolyte vapour pressure via battery testing calorimetery. Over-pressure builds up along with the programmed heating of the cell, and as a result, the thermal runaway is triggered at 20 to 45 K over the electrolyte boiling point, corresponding to 70 to 150 kPa pressure difference between the cell and the environment. The distinct performance-safety-cost behaviours of three ether type of electrolytes stems from the different CH2CH2O chain lengths. Such molecular insight will serve as a fundamental guideline in choosing and designing the desired electrolyte that simultaneously achieves a high explosion limit and good electrochemical performance.	Jan 2021

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