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Hélène
Ginestet
,
Rachel J.
Husband
,
Nicolas
Jaisle
,
Eric
Edmund
,
Zuzana
Konôpková
,
Cornelius
Strohm
,
Madden S.
Anae
,
Daniele
Antonangeli
,
Karen
Appel
,
Orianna B.
Ball
,
Marzena
Baron
,
Silvia
Boccato
,
Khachiwan
Buakor
,
Julien
Chantel
,
Hyunchae
Cynn
,
Anand P.
Dwivedi
,
Heinz
Graafsma
,
Egor
Koemets
,
Torsten
Laurus
,
Hauke
Marquardt
,
Bernhard
Massani
,
James D.
Mchardy
,
Malcolm I.
Mcmahon
,
Vitali
Prakapenka
,
Jolanta
Sztuk-Dambietz
,
Minxue
Tang
,
Tianqi
Xie
,
Zena
Younes
,
Ulf
Zastrau
,
Alexander F.
Goncharov
,
Clemens
Prescher
,
Agnes
Dewaele
,
R. Stewart
Mcwilliams
,
Guillaume
Morard
,
Sébastien
Merkel
Open Access
Abstract: The development of pulsed intense x-ray sources, such as free electron laser, offers new avenues for high pressure experiments. Here, we study the feasibility and metrology of x-ray heating in diamond anvil cells at the European x-ray free electron laser. This method enables one to volumetrically heat the sample while inhibiting chemical migration and probing the crystallographic structure of the sample throughout the heating with a high repetition rate. We focus our study on iron, whose phase diagram is well established up to 100 GPa, to explore the possibilities and limitations of this technique. We volumetrically heat iron samples at starting pressures ranging from 10 to 138 GPa, using the x-ray beam pulsed at 4.5 MHz in a serial pump-and-probe experimental design. Experimental challenges arise from temperature gradients within the sample, changes in temperature at the 100 ns timescale, the difficulty of direct temperature estimates, the effect of thermal pressure, and the presence of metastable crystallites due to rapid cycles of heating and cooling. Hence, we develop a multi-crystal-like data processing method that allows us to account for sample heterogeneity in probed conditions. We then calibrate our measurements using known physical properties of iron under pressure. Thermal pressure in our experiments increases from 4% of the isochoric prediction at 10 GPa to 23% at 138 GPa, and we show that our data are in agreement with most previous observations of iron in this pressure range. The method can now be implemented at higher pressures and temperatures and on materials with unknown phase diagrams.
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Jan 2026
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Detectors
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N.
Goyal
,
S.
Aplin
,
A.
Balerna
,
P.
Bell
,
J.
Casas
,
M.
Cascella
,
S.
Chatterji
,
C.
Cohen
,
E.
Collet
,
P.
Fajardo
,
E. N.
Gimenez
,
H.
Graafsma
,
H.
Hiresmann
,
F.j.
Iguaz
,
K.
Klementiv
,
K.
Kolodjiez
,
L.
Manzanillas
,
T.
Martin
,
R. H.
Menk
,
M.
Porro
,
M.
Quispe
,
B.
Schmitt
,
S.
Scully
,
M.
Turcato
,
C.
Ward
,
E.
Welter
Abstract: The XAFS-DET work package of the European LEAPS-INNOV project is developing high-purity Germanium detectors for synchrotron applications requiring spectroscopic-grade response. The detectors integrate three key features: (1) newly designed monolithic Germanium sensors optimised to mitigate charge-sharing events, (2) an improved cooling and mechanical design structure supported by thermal simulations, and (3) complete electronic chain featuring a low-noise CMOS technology based preamplifier, enabling high X-ray count rate capability over a broad energy range (5-100 keV). This paper discusses the first integration and characterization of one of the two multi-element Ge detectors at the European Synchrotron Radiation Facility (ESRF). The integration phase included validating high-throughput front-end electronics, integrating them with the Ge sensor, and operating them at liquid nitrogen temperature, in addition to the experimental characterization, which consists of electronics noise study and spectroscopic performance evaluation.
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Jul 2025
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Detectors
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E. N.
Gimenez
,
A.
Balerna
,
M.
Cascella
,
S.
Chatterji
,
C.
Cohen
,
P.
Fajardo
,
H.
Graafsma
,
N.
Goyal
,
H.
Hirsemann
,
F. J.
Iguaz
,
K.
Klementiev
,
T.
Kołodziej
,
T.
Martin
,
R. H.
Menk
,
M.
Porro
,
M.
Quispe
,
B.
Schmitt
,
S.
Scully
,
J.
Spiers
,
M.
Turcato
,
C.
Ward
,
E.
Welter
Open Access
Abstract: Recent upgrades in synchrotron radiation facilities, which now produce highly brilliant and coherent beams, result in a broader array of experiments challenging the available detectors. In X-ray Absorption Fine Structure (XAFS) experiments, detector performance is often a limiting factor, especially with the high photon fluxes from upgraded facilities. Within this context, a consortium of European facilities has joined under the LEAPS-INNOV project to push the current technologies and develop a germanium detector that can operate under high photon fluxes. The latest status of the XAFS detector development is presented here. The project has moved from the design and simulations phase to the assembled stage, with the sensor, electronic chain and mechanics being manufactured and tested. Next steps are focused on integrating all parts together and characterize the detector performance with X-ray beam.
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May 2025
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Detectors
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M.
Hajheidari
,
C. B.
Wunderer
,
J.
Correa
,
A.
Marras
,
S.
Lange
,
M.
Dahlgruen
,
J.
Gebert
,
F.
Krivan
,
I.
Shevyakov
,
V.
Vardanyan
,
Th.
Wendt
,
M.
Hoesch
,
K.
Bagschik
,
N.
Guerrini
,
B.
Marsh
,
I.
Sedgwick
,
T.
Nicholls
,
G.
Cautero
,
D.
Giuressi
,
R. H.
Menk
,
L.
Stebel
,
A.
Greer
,
W.
Nichols
,
M.
Nakhostin
,
H. J.
Hyun
,
K. S.
Kim
,
S. H.
Kim
,
S. Y.
Park
,
S. Y.
Rah
,
E.
Plönjes
,
G.
Brenner
,
K.
Kharitonov
,
F.
Goutierrez
,
T.
Hirono
,
M.
Ruiz-Lopez
,
R.
Pan
,
S.
Gang
,
B.
Keitel
,
S.
Jelinek
,
R.
Radloff
,
H.
Graafsma
Open Access
Abstract: Percival is a CMOS-based imager with 2 megapixels, also called P2M, designed for photon science experiments. The first generation of the P2M sensor showed some performance issues. Specifically, ADCs in full-speed operation mode are affected by crosstalk and show a non-linear and uncorrectable response. A firmware hack to the readout and data acquisition system has been introduced to partially overcome these effects, at the cost of limiting the frame rate to 83 Hz. Moreover, a non-uniform dark response of the sensor pixels is observed, explained by non-uniform bias currents across the chip: two opposite edges of the sensor cannot be digitized when applying biases that have the centre of the sensor operating normally. These issues are addressed in the re-submission of the chip. In this contribution, we present the current status of the detector and the first results from the re-designed sensor.
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May 2025
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Detectors
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N.
Goyal
,
S.
Aplin
,
A.
Balerna
,
P.
Bell
,
J.
Casas
,
M.
Cascella
,
S.
Chatterji
,
C.
Cohen
,
E.
Collet
,
G.
Dennis
,
P.
Fajardo
,
E. N.
Gimenez
,
H.
Graafsma
,
H.
Hiresmann
,
F. J.
Iguaz
,
K.
Klementiev
,
T.
Kolodziej
,
L.
Manzanillas
,
T.
Martin
,
R. H.
Menk
,
M.
Porro
,
M.
Quispe
,
B.
Schmitt
,
S.
Scully
,
M.
Turcato
,
C.
Ward
,
E.
Welter
Open Access
Abstract: This study presents a detailed simulation-based analysis of the detection limits of multi-element monolithic Germanium (Ge) detectors to cadmium traces in environmental soil samples. Using the capabilities of the Geant4 Monte Carlo toolkit in combination with the Solid State Detector Package, we evaluated the detection limit variation with the sample-to-detector distances and photon flux. These simulations were conducted to mimic realistic conditions, with a photon flux measured by the SAMBA beamline at the SOLEIL synchrotron facility. Our findings for the detection limit for trace amounts of pollutants in low concentrations like cadmium in the soil provide valuable insights for optimizing experimental setups in environmental monitoring and synchrotron-based applications, where precise detection of trace elements is critical.
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May 2025
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Detectors
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Francesco
Guzzi
,
Alessandra
Gianoncelli
,
Luigi
Stebel
,
Dario
Giuressi
,
Giuseppe
Cautero
,
Roberto
Borghes
,
Iztok
Gregori
,
Fulvio
Billè
,
Martin
Scarcia
,
Valentina
Bonanni
,
Milan
Žižić
,
Hyojung
Hyun
,
William
Nichols
,
Jonathan
Correa
,
Alessandro
Marras
,
Corenelia B.
Wunderer
,
Heinz
Graafsma
,
Ralf Hendrik
Menk
,
George
Kourousias
Open Access
Abstract: PERCIVAL is a novel soft X-ray detection system designed for the needs of modern microscopy. By integrating it into the TwinMic end-station at Elettra Sincrotrone Trieste, we conducted an exploratory computational microscopy experiment on biological samples, aiming at evaluating the entire system in a real use-case scenario. We present the methodology to convert the RAW data and our high-resolution image reconstructions.
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Jan 2025
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Detectors
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J.
Correa
,
M.
Mehrjoo
,
R.
Battistelli
,
F.
Lehmkühler
,
A.
Marras
,
C. B.
Wunderer
,
T.
Hirono
,
V.
Felk
,
F.
Krivan
,
S.
Lange
,
I.
Shevyakov
,
V.
Vardanyan
,
M.
Zimmer
,
M.
Hoesch
,
K.
Bagschik
,
N.
Guerrini
,
B.
Marsh
,
I.
Sedgwick
,
G.
Cautero
,
L.
Stebel
,
D.
Giuressi
,
R. H.
Menk
,
A.
Greer
,
T.
Nicholls
,
W.
Nichols
,
U.
Pedersen
,
P.
Shikhaliev
,
N.
Tartoni
,
H. J.
Hyun
,
S. H.
Kim
,
S. Y.
Park
,
K. S.
Kim
,
F.
Orsini
,
F. J.
Iguaz
,
F.
Büttner
,
B.
Pfau
,
E.
Plönjes
,
K.
Kharitonov
,
M.
Ruiz-Lopez
,
R.
Pan
,
S.
Gang
,
B.
Keitel
,
H.
Graafsma
Open Access
Abstract: The PERCIVAL detector is a CMOS imager designed for the soft X-ray regime at photon sources. Although still in its final development phase, it has recently seen its first user experiments: ptychography at a free-electron laser, holographic imaging at a storage ring and preliminary tests on X-ray photon correlation spectroscopy. The detector performed remarkably well in terms of spatial resolution achievable in the sample plane, owing to its small pixel size, large active area and very large dynamic range; but also in terms of its frame rate, which is significantly faster than traditional CCDs. In particular, it is the combination of these features which makes PERCIVAL an attractive option for soft X-ray science.
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Jan 2023
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Detectors
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L.
Manzanillas
,
S.
Aplin
,
A.
Balerna
,
P.
Bell
,
J.
Casas
,
M.
Cascella
,
S.
Chatterji
,
C.
Cohen
,
G.
Dennis
,
P.
Fajardo
,
H.
Graafsma
,
H.
Hirsemann
,
F. J.
Iguaz
,
K.
Klementiev
,
T.
Kołodziej
,
T.
Martin
,
R.
Menk
,
F.
Orsini
,
M.
Porro
,
M.
Quispe
,
B.
Schmitt
,
N.
Tartoni
,
M.
Turcato
,
C.
Ward
,
E.
Welter
Abstract: In past years efforts have concentrated on the development of arrays of Silicon Drift Detectors for X-ray spectroscopy. This is in stark contrast to the little effort that has been devoted to the improvement of germanium detectors, in particular for synchrotron applications. Germanium detectors have better energy resolution and are more efficient in detecting high energy photons than silicon detectors. In this context, the detector consortium of the European project LEAPS-INNOV has set an ambitious R&D program devoted to the development of a new generation of multi-element monolithic germanium detectors for X-ray detection. In order to improve the performance of the detector under development, simulations of the different detector design options have been performed. In this contribution, the efforts in terms of R&D are outlined with a focus on the modelization of the detector geometry and first performance results. These performance results show that a signal-to-background ratio larger than 1000 can be achieved in the energy range of interest from 5 keV to 100 keV.
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Dec 2022
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Detectors
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F.
Orsini
,
S.
Aplin
,
A.
Balerna
,
P.
Bell
,
J.
Casas
,
M.
Cascella
,
S.
Chatterji
,
C.
Cohen
,
G.
Dennis
,
P.
Fajardo
,
H.
Graafsma
,
H.
Hirsemann
,
F. J.
Iguaz
,
K.
Klementiev
,
T.
Kołodziej
,
L.
Manzanillas
,
T.
Martin
,
R.
Menk
,
M.
Porro
,
M.
Quispe
,
B.
Schmitt
,
N.
Tartoni
,
M.
Turcato
,
C.
Ward
,
E.
Welter
Abstract: The high brilliance and coherent beams resulting from recent upgraded synchrotron radiation facilities open the way for a large range of experiments, where detectors play a key role in the techniques and methods developed to fully exploit the upgraded synchrotron. For instance, one of the major limitations of XAFS experiment is the performance of the detectors. In order to be able to measure more challenging samples and to cope with the very high photon flux of the current and future (diffraction limited) sources, technological developments of detectors are necessary. In this framework, the germanium detector developed in the European project LEAPS-INNOV aims at improving several technological aspects. This type of detector represents a very important class of instruments for X-ray spectroscopy due to the fact that they enable to detect efficiently photons of considerable higher energy with respect to silicon detectors. The objective of this project consists in pushing the detector performance beyond the state-of-the-art. Preliminary layout and main choices for the design studies of this new detector are presented in this paper.
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Oct 2022
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Detectors
|
Alessandro
Marras
,
Jonathan
Correa
,
Sabine
Lange
,
Vahagn
Vardanyan
,
Tim
Gerhardt
,
Manuela
Kuhn
,
Frantisek
Krivan
,
Igor
Shevyakov
,
Manfred
Zimmer
,
Moritz
Hoesch
,
Kai
Bagschik
,
Frank
Scholz
,
Niccolo
Guerrini
,
Ben
Marsh
,
Iain
Sedgwick
,
Giuseppe
Cautero
,
Dario
Giuressi
,
Gregori
Iztok
,
Ralf H.
Menk
,
Martin
Scarcia
,
Luigi
Stebel
,
Tim
Nicholls
,
William
Nichols
,
Ulrik K.
Pedersen
,
Polad
Shikhaliev
,
Nicola
Tartoni
,
Hyojung
Hyun
,
Seonghan
Kim
,
Kyungsook
Kim
,
Seungyu
Rah
,
Arkadiusz
Dawiec
,
Fabienne
Orsini
,
Giovanni
Pinaroli
,
Alan
Greer
,
Steve
Aplin
,
April D.
Jewell
,
Todd J.
Jones
,
Shouleh
Nikzad
,
Michael E.
Hoenk
,
Frank
Okrent
,
Heinz
Graafsma
,
Cornelia B.
Wunderer
Open Access
Abstract: In this paper the back-side-illuminated Percival 2-Megapixel (P2M) detector is presented, along with its characterization by means of optical and X-ray photons. For the first time, the response of the system to soft X-rays (250 eV to 1 keV) is presented. The main performance parameters of the first detector are measured, assessing the capabilities in terms of noise, dynamic range and single-photon discrimination capability. Present limitations and coming improvements are discussed.
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Jan 2021
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