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Instruments / Technical Area	Publication Details	Published	Actions
B23-Circular Dichroism I02-Macromolecular Crystallography	Guanine can direct binding specificity of Ru-dppz complexes to DNA through steric effects James Pearce Hall , Sarah Prava Gurung , Jessica Henle , Patrick Poidl , Johanna Andersson , Per Lincoln , Graeme Winter , Thomas Sorensen , David John Cardin , John Brazier , Christine J Cardin Chemistry - A European Journal DOI: 10.1002/chem.201605508 Diamond Proposal Number(s): [9078, 7597, 15733] Open Access Show Abstract ▼ Abstract: X-ray crystal structures of three Λ-[Ru(L)2dppz]2+ complexes (L=phen, bpy) bound to d((5BrC)GGC/GCCG) show the compounds intercalated at a 5´-CG-3´ step. The compounds bind through canted intercalation, with the binding angle determined by the guanine-NH2 group, in contrast to symmetrical intercalation previously observed at 5´-TA-3´ sites. This result suggests that canted intercalation is preferred at 5´-CG-3´ sites even though the site itself is symmetrical, and we hypothesise that symmetrical intercalation in a 5´-CG-3´ step could give rise to a longer luminescence lifetime than canted intercalation.	Jan 2017

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