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Instruments / Technical Area	Publication Details	Published
I05-ARPES	Surface states and Rashba-type spin polarization in antiferromagnetic MnBi2Te4(0001) R. C. Vidal , H. Bentmann , T. R. F. Peixoto , A. Zeugner , S. Moser , C.-h. Min , S. Schatz , K. Kissner , M. Unzelmann , C. I. Fornari , H. B. Vasili , M. Valvidares , K. Sakamoto , D. Mondal , J. Fujii , I. Vobornik , S. Jung , C. Cacho , T. K. Kim , R. J. Koch , C. Jozwiak , A. Bostwick , J. D. Denlinger , E. Rotenberg , J. Buck , M. Hoesch , F. Diekmann , S. Rohlf , M. Kalläne , K. Rossnagel , M. M. Otrokov , E. V. Chulkov , M. Ruck , A. Isaeva , F. Reinert Physical Review B 100, 121104(R) DOI: 10.1103/PhysRevB.100.121104 Diamond Proposal Number(s): [19278, 22468] Show Abstract ▼ Abstract: The layered van der Waals antiferromagnet MnBi 2 Te 4 has been predicted to combine the band ordering of archetypical topological insulators such as Bi 2 Te 3 with the magnetism of Mn, making this material a viable candidate for the realization of various magnetic topological states. We have systematically investigated the surface electronic structure of MnBi 2 Te 4 (0001) single crystals by use of spin- and angle-resolved photoelectron spectroscopy experiments. In line with theoretical predictions, the results reveal a surface state in the bulk band gap and they provide evidence for the influence of exchange interaction and spin-orbit coupling on the surface electronic structure.	Sep 2019
I05-ARPES	Magnetic Weyl semimetal phase in a Kagomé crystal D. F. Liu , A. J. Liang , E. K. Liu , Q. N. Xu , Y. W. Li , C. Chen , D. Pei , W. J. Shi , S. K. Mo , P. Dudin , T. Kim , C. Cacho , G. Li , Y. Sun , L. X. Yang , Z. K. Liu , S. S. P. Parkin , C. Felser , Y. L. Chen Science 365, 1282 - 1285 DOI: 10.1126/science.aav2873 Diamond Proposal Number(s): [22367, 20683] Show Abstract ▼ Abstract: Weyl semimetals are crystalline solids that host emergent relativistic Weyl fermions and have characteristic surface Fermi-arcs in their electronic structure. Weyl semimetals with broken time reversal symmetry are difficult to identify unambiguously. In this work, using angle-resolved photoemission spectroscopy, we visualized the electronic structure of the ferromagnetic crystal Co3Sn2S2 and discovered its characteristic surface Fermi-arcs and linear bulk band dispersions across the Weyl points. These results establish Co3Sn2S2 as a magnetic Weyl semimetal that may serve as a platform for realizing phenomena such as chiral magnetic effects, unusually large anomalous Hall effect and quantum anomalous Hall effect.	Sep 2019
I05-ARPES	Nanoscale mapping of quasiparticle band alignment Soeren Ulstrup , Cristina E. Giusca , Jill A. Miwa , Charlotte Sanders , Alex Browning , Pavel Dudin , Cephise Cacho , Olga Kazakova , D. Kurt Gaskill , Rachael L. Myers-ward , Tianyi Zhang , Mauricio Terrones , Philip Hofmann Nature Communications 10 DOI: 10.1038/s41467-019-11253-2 Diamond Proposal Number(s): [19260] Open Access Show Abstract ▼ Abstract: Control of atomic-scale interfaces between materials with distinct electronic structures is crucial for the design and fabrication of most electronic devices. In the case of two-dimensional materials, disparate electronic structures can be realized even within a single uniform sheet, merely by locally applying different vertical gate voltages. Here, we utilize the inherently nano-structured single layer and bilayer graphene on silicon carbide to investigate lateral electronic structure variations in an adjacent single layer of tungsten disulfide (WS2). The electronic band alignments are mapped in energy and momentum space using angle-resolved photoemission with a spatial resolution on the order of 500 nm (nanoARPES). We find that the WS2 band offsets track the work function of the underlying single layer and bilayer graphene, and we relate such changes to observed lateral patterns of exciton and trion luminescence from WS2.	Jul 2019
I05-ARPES	Chiral topological semimetal with multifold band crossings and long Fermi arcs Niels B. M. Schröter , Ding Pei , Maia G. Vergniory , Yan Sun , Kaustuv Manna , Fernando De Juan , Jonas A. Krieger , Vicky Süss , Marcus Schmidt , Pavel Dudin , Barry Bradlyn , Timur K. Kim , Thorsten Schmitt , Cephise Cacho , Claudia Felser , Vladimir N. Strocov , Yulin Chen Nature Physics 353 DOI: 10.1038/s41567-019-0511-y Diamond Proposal Number(s): [19883, 21400] Show Abstract ▼ Abstract: Topological semimetals in crystals with a chiral structure (which possess a handedness due to a lack of mirror and inversion symmetries) are expected to display numerous exotic physical phenomena, including fermionic excitations with large topological charge1, long Fermi arc surface states2,3, unusual magnetotransport4 and lattice dynamics5, as well as a quantized response to circularly polarized light6. So far, all experimentally confirmed topological semimetals exist in crystals that contain mirror operations, meaning that these properties do not appear. Here, we show that AlPt is a structurally chiral topological semimetal that hosts new four-fold and six-fold fermions, which can be viewed as a higher spin generalization of Weyl fermions without equivalence in elementary particle physics. These multifold fermions are located at high symmetry points and have Chern numbers larger than those in Weyl semimetals, thus resulting in multiple Fermi arcs that span the full diagonal of the surface Brillouin zone. By imaging these long Fermi arcs, we experimentally determine the magnitude and sign of their Chern number, allowing us to relate their dispersion to the handedness of their host crystal.	May 2019
I05-ARPES	Buried double CuO chains in YBa2Cu4O8 uncovered by nano-ARPES Hideaki Iwasawa , Pavel Dudin , Kyosuke Inui , Takahiko Masui , Timur K. Kim , Cephise Cacho , Moritz Hoesch Physical Review B 99 DOI: 10.1103/PhysRevB.99.140510 Diamond Proposal Number(s): [21083] Show Abstract ▼ Abstract: Identifying the electron dynamics in CuO chains has been elusive in Y-Ba-Cu-O (YBCO) cuprate systems when using standard angle-resolved photoemission spectroscopy (ARPES); a cleaved sample exhibits areas terminated by both CuO chains or BaO layers, and the size of a typical beam results in ARPES signals that are superposed from both terminations. Here, we employ spatially resolved ARPES with a submicrometric beam (nano-ARPES) to reveal the surface-termination-dependent electronic structures of the double CuO chains in YBa 2 Cu 4 O 8 . We present an observation of sharp metallic dispersions and Fermi surfaces of the double CuO chains buried underneath the CuO 2 -plane block on a BaO-terminated surface. While the observed Fermi surfaces of the CuO chains are highly one dimensional, the electrons in the CuO chains do not undergo significant electron correlations and no signature of a Tomonaga-Luttinger liquid or a marginal Fermi liquid is found. Our work represents an important experimental step toward understanding the charge dynamics and provides a starting basis for modeling the high- T c superconductivity in YBCO cuprate systems.	Apr 2019

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