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Instruments / Technical Area	Publication Details	Published	Actions
I22-Small angle scattering & Diffraction	Designing and controlling transient supramolecular gels Dave J. Adams , Emma Bowley , Simona Bianco , Fin Hallam Stewart , Chloe Wallace , Rebecca Ginesi , Alex Loch , Martin Rosenthal , Andrew Smith Chemsystemschem DOI: 10.1002/syst.202400073 Diamond Proposal Number(s): [32866] Open Access Show Abstract ▼ Abstract: Supramolecular systems are often designed such that a steady state exists. However, the ability to design systems with pre-determined changes in state can lead to highly dynamic materials, with evolving supramolecular structures and adaptable material properties. This approach is of great interest from the perspective of designing adaptive systems as well as from a broader systems chemistry perspective. Here, we report how a transient system can be altered to access different mechanical properties and transitions by varying the trigger and temperature. The aging of these systems is also explored, as the networks continually evolve long past the common cut-off point of analysis of one day. We therefore provide new insights into the control of transient gels, as well as an understanding as to the underpinning supramolecular structures and how they evolve with time.	Nov 2024
I22-Small angle scattering & Diffraction	Controlling self‐sorting versus co‐assembly in supramolecular gels Santanu Panja , Bart Dietrich , Andrew Smith , Annela Seddon , Dave J. Adams Chemsystemschem DOI: 10.1002/syst.202200008 Diamond Proposal Number(s): [27906] Open Access Show Abstract ▼ Abstract: Supramolecular gels formed by the combination of different organic molecules are of significant interest in the search of new functional materials. When two different molecules are mixed to form gels, the self-assembled fibres can be a result of self-sorting or co-assembly. A key challenge is to control the network type. Here, we demonstrate that control over the network type can be achieved either by varying the hydrophobicity of a component or by employing a pH-switch method.	Mar 2022

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