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Instruments / Technical Area	Publication Details	Published	Actions
I09-Surface and Interface Structural Analysis	Modifying the surface of a Rashba-split Pb-Ag alloy using tailored metal-organic bonds Benjamin Stadtmueller , Johannes Seidel , Norman Haag , Lisa Grad , Christian Tusche , Gerben Van Straaten , Markus Franke , Jürgen Kirschner , Christian Kumpf , Mirko Cinchetti , Martin Aeschlimann Physical Review Letters 117, 096805 DOI: 10.1103/PhysRevLett.117.096805 Diamond Proposal Number(s): [10370, 11915] Show Abstract ▼ Abstract: Hybridization-related modifications of the first metal layer of a metal-organic interface are difficult to access experimentally and have been largely neglected so far. Here, we study the influence of specific chemical bonds (as formed by the organic molecules CuPc and PTCDA) on a Pb-Ag surface alloy.We find that delocalized van der Waals or weak chemical π-type bonds are not strong enough to alter the alloy, while localized σ-type bonds lead to a vertical displacement of the Pb surface atoms and to changes in the alloy’s surface band structure. Our results provide an exciting platform for tuning the Rashba-type spin texture of surface alloys using organic molecules.	Aug 2016

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