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Selective Adsorption of Sulfur Dioxide in a Robust Metal-Organic Framework Material

DOI: 10.1002/adma.201602338 DOI Help

Authors: Mathew Savage (School of Chemistry, University of Manchester) , Yongqiang Cheng (The Chemical and Engineering Materials Division (CEMD), Neutron Sciences Directorate, Oak Ridge National Laboratory) , Timothy L. Easun (School of Chemistry, Cardiff University, Cardiff) , Jennifer E. Eyley (School of Chemistry, University of Manchester) , Stephen P. Argent (School of Chemistry, University of Nottingham) , Mark Warren (Diamond Light Source) , William Lewis (School of Chemistry, University of Nottingham) , Claire Murray (Diamond Light Source) , Chiu C. Tang (Diamond Light Source) , Mark D. Frogley (Diamond Light Source) , Gianfelice Cinque (Diamond Light Source) , Junliang Sun (College of Chemistry and Molecular Engineering, Peking University) , Svemir Rudić (ISIS Neutron & Muon Source, STFC Rutherford Appleton Laboratory) , Richard T. Murden (Hiden Isochema, Warrington) , Michael J. Benham (Hiden Isochema, Warrington) , Andrew N. Fitch (European Synchrotron Radiation Facility) , Alexander J. Blake (School of Chemistry, University of Nottingham) , Anibal J. Ramirez-cuesta (The Chemical and Engineering Materials Division (CEMD), Neutron Sciences Directorate, Oak Ridge National Laboratory) , Sihai Yang (School of Chemistry, University of Manchester) , Martin Schröder (School of Chemistry, University of Manchester)
Co-authored by industrial partner: No

Type: Journal Paper
Journal: Advanced Materials

State: Published (Approved)
Published: August 2016
Diamond Proposal Number(s): 9444 , 5839 , 12516

Open Access Open Access

Abstract: Selective adsorption of SO2 is realized in a porous metal–organic framework material, and in-depth structural and spectroscopic investigations using X-rays, infrared, and neutrons define the underlying interactions that cause SO2 to bind more strongly than CO2 and N2.

Journal Keywords: metal–organic frameworks;sulfur dioxide;carbon dioxide;indium;carboxylates

Subject Areas: Materials


Instruments: B22-Multimode InfraRed imaging And Microspectroscopy , I11-High Resolution Powder Diffraction , I19-Small Molecule Single Crystal Diffraction

Documents:
Savage_et_al-2016-Advanced_Materials.pdf