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Coherent orbital waves in the photo-induced insulator–metal dynamics of a magnetoresistive manganite

DOI: 10.1038/nmat1979 DOI Help

Authors: D. Polli (Politecnico di Milano, Italy) , M. Rini (Lawrence Berkeley National Laboratory, USA) , Simon Wall (University of Oxford) , R. W. Schoenlein (Lawrence Berkeley National Laboratory, USA) , Y. Tomioka (Correlated Electron Research Center, Japan) , Y. Tokura (Correlated Electron Research Center, Japan) , G. Cerullo (Politecnico di Milano, Italy) , Andrea Cavalleri (University of Oxford & Diamond Light Source)
Co-authored by industrial partner: No

Type: Journal Paper
Journal: Nature Materials , VOL 6 (9) , PAGES 643 - 647

State: Published (Approved)
Published: August 2007

Abstract: Photo-excitation can drive strongly-correlated electron insulators into competing conducting phases, resulting in giant and ultrafast changes of their electronic and magnetic properties. The underlying non-equilibrium dynamics involve many degrees of freedom at once, whereby sufficiently short optical pulses can trigger the corresponding collective modes of the solid along temporally coherent pathways. Their characteristic frequencies of these modes range between the few GHz of acoustic vibrations to the tens or even hundreds of THz for purely electronic excitations. Virtually all experiments to date have used 100-fs or longer pulses, detecting only comparatively slow lattice dynamics. Here, we use sub-10-fs optical pulses to study the photo-induced insulator-metal transition in the magneto-resistive manganite Pr0.7Ca0.3MnO3. At room temperature, we find that the time-dependent pathway toward the metallic phase is accompanied by coherent 31-THz oscillations of the optical reflectivity, significantly faster than all lattice vibrations. These high-frequency oscillations are suggestive of coherent orbital waves, crystal-field excitations triggered here by Impulsive Stimulated Raman Scattering. Orbital waves are likely to be initially localized to the small polarons of this room-temperature manganite, coupling to other degrees of freedom at longer times and seeding the coalescence of photo-domains into a metallic phase.

Subject Areas: Physics


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