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Crystallisation in basaltic magmas revealed via in situ 4D synchrotron X-ray microtomography
DOI:
10.1038/s41598-018-26644-6
Authors:
M.
Polacci
(University of Manchester)
,
F.
Arzilli
(University of Manchester)
,
G.
La Spina
(University of Manchester)
,
N.
Le Gall
(University of Manchester)
,
B.
Cai
(University of Manchester)
,
M. E.
Hartley
(University of Manchester)
,
D.
Di Genova
(University of Bristol)
,
Nghia
Vo
(Diamond Light Source)
,
S.
Nonni
(University of Manchester Harwell Campus)
,
R. C.
Atwood
(Diamond Light Source)
,
E. W.
Llewellin
(Durham University)
,
P. D.
Lee
(University of Manchester)
,
M. R.
Burton
(University of Manchester)
Co-authored by industrial partner:
No
Type:
Journal Paper
Journal:
Scientific Reports
, VOL 8
State:
Published (Approved)
Published:
May 2018
Diamond Proposal Number(s):
12392
,
16188

Abstract: Magma crystallisation is a fundamental process driving eruptions and controlling the style of volcanic activity. Crystal nucleation delay, heterogeneous and homogeneous nucleation and crystal growth are all time-dependent processes, however, there is a paucity of real-time experimental data on crystal nucleation and growth kinetics, particularly at the beginning of crystallisation when conditions are far from equilibrium. Here, we reveal the first in situ 3D time-dependent observations of crystal nucleation and growth kinetics in a natural magma, reproducing the crystallisation occurring in real-time during a lava flow, by combining a bespoke high-temperature environmental cell with fast synchrotron X-ray microtomography. We find that both crystal nucleation and growth occur in pulses, with the first crystallisation wave producing a relatively low volume fraction of crystals and hence negligible influence on magma viscosity. This result explains why some lava flows cover kilometres in a few hours from eruption inception, highlighting the hazard posed by fast-moving lava flows. We use our observations to quantify disequilibrium crystallisation in basaltic magmas using an empirical model. Our results demonstrate the potential of in situ 3D time-dependent experiments and have fundamental implications for the rheological evolution of basaltic lava flows, aiding flow modelling, eruption forecasting and hazard management.
Journal Keywords: Petrology; Volcanology
Diamond Keywords: Volcanology
Subject Areas:
Earth Science
Instruments:
I12-JEEP: Joint Engineering, Environmental and Processing
Added On:
31/05/2018 08:50
Documents:
s41598-018-26644-6.pdf
Discipline Tags:
Earth Sciences & Environment
Natural disaster
Geology
Geochemistry
Technical Tags:
Imaging
Tomography